written by Prof. Akira SATOH

on 1st of January, 2012
Results between 2011 and today





1.  Behavior of Magnetic Particles in a Flow between the Parallel Walls by Means of the Lattice Boltzmann Method 




We have investigated the behavior of magnetic particles between the
two parallel walls in a non-uniform applied magnetic field situation.
 
Magnetic particles will move into the region on this macroscopic flow
through the upstream boundary surface, be attracted around each
magnetic pole under the non-equilibrium magnetic field, or move in
the downstream direction without being attracted, and move out of
the simulation area thorough the downstream surface.


This simulation may be an advancing simulation in which the Brownian motion is activated by means of the viscosity-modified
procedure and the multi-body hydrodynamic interactions are taken into account. 




For the case where the magnetic field is more dominant
than the magnetic interaction between particles, 
magnetic particles are attracted to the wall surface
around the magnetic poles to form short chain-like
clusters from the attached particles.

For the case where the magnetic field is equal to the
influence of the magnetic interaction between particles,
 some clusters are formed in a loop-like formation and
move in the downstream direction without attachment to
the magnetic poles and some clusters are formed in a
long chain-like formation with the end particles anchored
around the magnetic pole.

For the case where the magnetic interaction between
particles is significantly dominant, large packed clusters
and chain-like clusters are formed and flow in the
downstream direction without attachment to the
magnetic poles. 






The magnetic particles flow in the center area except
for a few layers of the particle diameter from the wall
surfaces, since the magnetic particles are attached
around the magnetic poles.











2.  Development of the Method of Activating the Particle Brownian Motion
in the Lattice Boltzmann Method

 

In order to apply the lattice Boltzmann method to a flow problem of magnetic suspensions, we
have investigated the feasibility of the viscosity-modifying method that is expected to be a technique
for sophisticating the activating method of the particle Brownian motion based on fluctuation
hydrodynamics.



The figures on the left-hand side are for a very weak applied
magnetic field and those on the right-hand side are for a very
strong applied magnetic field.

The snapshots at a lower position are obtained for a stronger
applied magnetic field. 

 
In the case of a weak magnetic field, network-like clusters are formed, and in the case of a strong magnetic field, chain-like clusters are formed in the magnetic field direction.  These aggregate structures are in good agreement with those of the Monte Carlo method. 








The figure shows the dependence of the heights of the first and second peaks of the pair correlation function on the volumetric fraction for the three cases of the particle diameter.

It is seen that the heights of the first and second peaks is in good agreement with that of the Monte Carlo method irrespective of the particle diameter.









We may conclude that the lattice Boltzmann method with the viscosity-scaling procedure is quite a possible technique for simulating a flow problem of magnetic particles under a non-uniform applied magnetic field.



 

The modified viscosity is almost constant and independent of the strengths of magnetic particle-field and particle-particle interactions, and the variation of the volumetric fraction.












3. Theoretical Analysis of the Behavior of Oblate Hematite Particles in
a Simple Shear Flow by Means of the Orientational Distribution Function




As a model of the oblate hematite particles that are generated experimentally, we use the oblate spheroidal particle shown in Fig.1. The particle is assumed to have a magnetic moment normal to the particle axis at the particle center. 











The orientational distribution of the oblate hematite particle comes to have a one-peak type shape.



The peak becomes sharper with increasing magnetic field strength.



The distributions at a lefter position are for a weak shear flow, and those at a lower position are for a stronger magnetic field.

















A larger apparent viscosity can be obtained for a stronger magnetic field and for a weaker shear flow.
.












An oblate particle with a larger aspect ratio leads to a larger apparent viscosity. 

















The quantity employed as an ordinate is seen to yield the same curve for the different values of the particle aspect ratio.


The diffusion coefficient has a strong relationship with the magnetic field strength.











4. Influence of the Spin Rotational Brownian Motion on the Negative
Magneto-Rheological Effect of Rod-like Hematite Particle Suspensions






As a model of the rod-like hematite particles, we use the prolate spheroidal particle shown in Fig.1. The particle is assumed to have a magnetic moment normal to the particle axis at the particle center. 













The orientational distribution has a one-peak type shape for a weak magnetic field, and comes to have a linear-peak type shape with increasing magnetic field strength.


(a) For a significantly weak magnetic field

One-peak type distribution.









(b) For a magnetic field with medium field strength








(c) For a significantly strong magnetic field

A linear-peak type shape









The spin rotational Brownian motion does not influence the shape of the orientational distribution.







The viscosity becomes NEGATIVE with increasing applied magnetic field strength as predicted by the theory without the
spin rotational Brownian motion. 

The spin rotational Brownian motion has a quantitative effect on
the negative viscosity, although the dependence of the negative
viscosity on the magnetic field strength is in qualitatively good
agreement with that of the theory without the spin rotational
Brownian motion

The effect of the spin rotational Brownian motion quantitatively
appears as a significant decrease in the negative viscosity
effect. 






The negative magneto-rheological effect can be obtained for
a larger aspect ratio or for a more prolate hematite particle.














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